Studies of immune response by antigen loaded biodegradable polymer particles

 
Principal Investigator :  Amulya K Panda

Project Associates / Assistants
ANS Eshwari
Anshu Richhariya
Ruchi Chube

Ph D Students
Yogesh K Katare
Surinder Mohan Singh

Collaborators
Ayub Quadri
Lalit C Garg
Om Singh
Pramod Upadhyay
Rahul Pal
SP Vyas, DHG Vishwavidyalaya, Sagar
Shantha Biotechnics Pvt Ltd, Hyderabad

The theme of the project is to evaluate the immunostimulatory activities associated with polymer entrapped antigens such as Tetanus Toxoid (TT), Hepatitis B surface antigen (HBsAg) and plasmid DNA expressing antigens for development of single shot vaccines. The main objective is to study the immune response from biodegradable polymer particles entrapping antigens and plasmid DNA. Immune responses from polymer particles entrapping TT, HBsAg or plasmid DNA expressing HBsAg protein will be evaluated to (i) develop single shot vaccination for TT and extension of such immunization approach for Hepatitis B surface antigen (HBsAg), (ii) analyse the immune response from antigen loaded particles by employing different polymer composition, particle size and usage of various immunization protocols; evaluate long term memory response using polymer particles base immunization; generate cell mediated immune response using antigen entrapped polymer particles, (iii) induce immune responses by polymer entrapped plasmid DNA expressing protein.

A.    Immune response with polymer entrapped TT particles

Parameters which influence the immunogenicity of polymer entrapped TT particles were investigated in detail. Apart from protection of immunoreactivity of antigen during particles formulation, the other parameter which influences the immuniogenicity are, size of the particles, loading of antigen and doses of antigen. These above three parameter were extensively evaluated using polymer entrapped TT particles in single doses. It was repeatedly observed that use of alum along with particles improved the antibody titers in Wistar rats. Thus all immunization studies were carried out with admixture of polymer particles and alum for development of single dose vaccine. It was observed that higher size particles (> 100 µm) elicited very low level of immune response. High anti-TT antibody titers were achieved as the size of the particles reduced from 40 to 4 µm. Nanoparticles (<1 µm size) helped in eliciting very early antibody response but the titers dropped within two months time. Particles size of 2-5 µm not only gave very high anti –TT antibody titers but also for a longer period of time from single point immunization. Immune response from particles having different loading of antigen do not gave rise to different titers upon single point immunization. Dose response studies with very low dose of TT in particles were carried to evaluate the immuno-stimulatory potential of particle based immunization. It was observed that at lower doses (5 to 1 lf TT), particles based immunization with alum generated higher antibody titers than the alum base immunization. Use of alum along with antigen entrapped polymer particles not only improve the initial antibody titers very rapidly but also helped in maintaining high antibody titer throughout the post immunization period. Adsorption studies of TT on to alum in presence of dummy polymer particles, its in vitro release and in vivo evaluation are under progress to understand mechanism of alum on improving immune response from polymer entrapped antigen.

Rats immunized with polymer entrapping TT particles were boosted with 0.5 lf of saline TT after a period of eight months to evaluate the secondary responses. It was observed that secondary immune responses generated after boosting was higher in groups of animal immunized with particles in comparison to alum adsorbed TT group. Secondary immune response from particles based immunization having different doses, loading and size were evaluated. Among different particles formulation, the ones which gave high initial primary response gave very high secondary antibody response upon boosting with soluble antigen. Even very low amount of entrapped TT (1 lf) from single point immunization gave rise to very high secondary immune response in comparison to the alum based immunization. Secondary immune response from polymer entrapped antigen was five times higher than that observed for alum adsorbed TT. These results indicated that particles base immunization results in improved immunological memory in comparison to alum based immunization. Experiments involving cytokines profile of primed T cells, affinity of antibody generated after boosting are under investigation to have better understanding of the high secondary response generated from particles base immunization.

B.        Development of single dose vaccine for HBsAg

Polymer particles entrapping HBsAg in PLA particles were evaluated for generation of antibody response. The aim was to develop single dose HBsAg vaccine using polymer particles, which can be an alternative to the three-dose vaccination schedule. Rats were immunized with different polymer formulation and doses and antibody titers were compared with three doses of HBsAg injection on alum. The seroprotective nature of HBsAg antibody generated from polymer particle base immunization were evaluated using AUSAB Kit (Abbot Lab, USA). For more than 9 months particles based immunization resulted in > 50 000 mIU/ml of HBsAg antibody titers. Antibody titer obtained from three injection of alum adsorbed HBsAg was however higher (170,000 mIU/ml) than single dose particle base immunization. However the polymer particles base immunization resulted in generation of bio-neutralizing antibody titer higher than the desired units required for sero-protection (10 mIU/ml). Immunization studies with different doses of polymer entrapped antigens (preferably lower doses) and pulsed release formulation to mimic the conventional immunization schedule are under progress. Secondary immune response generated from immunization with polymer entrapped antigen was compared with three injection schedule of alum adsorbed HBsAg. Animals were boosted with 2 mg of soluble HBsAg after 9 months of post immunization and the antibody titers were evaluated. Very high anti-HBsAg titers (400,000 mIU/ml) were achieved within 15-20 days of post booster injection both for polymer entrapped as well alum adsorbed immunization. This indicated that single dose of polymer entrapped antigen is equally suitable to the three dose alum adsorbed HBsAg immunization for generation of high secondary immune response. Polymer entrapped HBsAg probably helps in generation of immunological memory as reported for tetanus immunization.

C.        Immunization of Plasmid DNA vaccine using polymer particles

Formulation and entrapment of HBsAg plasmid DNA in polymer matrix have been attempted to develop single dose DNA vaccine. Currently we are developing large-scale plasmid DNA preparation methods for immunization. We have been able to develop an improved process for the purification of pharmaceutical grade plasmid DNA for immunization process. The new method does not use ultracentrifugation, RNAse addition or column chromatography steps for the purification of plasmid DNA. From shaker flask culture, 2-3 mg of pure plasmid free from RNA and having negligible amount of endotoxin could be achieved. Pure plasmid yields are comparable to that of plasmid preparation using commercially available purification column. Process optimization studies combining high cell density fermentation and purification are under investigation to produce 10-20 mg pure plasmid from one litre of bacterial culture.

Publications

Original peer-reviewed articles

1.     Raghuvanshi RS, Singh O and Panda AK (2002) Correlation between in vitro release and in vivo immune response from biodegradable polymer particles entrapping tetanus toxoid. Drug Delivery 9:113-120.

2.     Raghuvanshi RS, Katare Y, Lalwani K, Ali MM, Singh O and Panda AK (2002) Improved immune response from biodegradable polymer particles entrapping tetanus toxoid by use of different immunization protocols and adjuvants. Int J Phram 245: 109-121.

3.     Gupta V, Eshwari ANS, Panda AK and Aggarwal GP (2002) Optimization of IMAC for single step purification of recombinant ovine growth hormone from inclusion bodies of E.coli. J Chromatogr (in press).

Reviews/Proceedings

1.     Panda AK (2002) Biochemical Engineering. In: CBSE book on Biotechnology. (Ed. Kannan K) CBSE Publication, New Delhi.

2.     Panda AK (2003) Bioprocessing of therapeutic protein from the inclusion bodies of E.coli In: Advances in biochemical engineering/biotechnology (Ed. Ghose TK) Springer Verlag,Germany (in press).

Patents

1.     Panda AK and Katare YK (2002) A process for developing immunological memory from single point immunization Indian patent application no. 754/DEL/2002.

2.     Panda AK, Sheikh GB, Eshwari ANS and Garg LC (2002) A process for solubilization and refolding of inclusion body. Indian patent application no. 921/DEL/2002 filed in Sep 2002.